Towards shot-noise limited diffraction experiments with table-top femtosecond hard x-ray sources

نویسندگان

  • Marcel Holtz
  • Christoph Hauf
  • Jannick Weisshaupt
  • Antonio-Andres Hernandez Salvador
  • Michael Woerner
  • Thomas Elsaesser
چکیده

Table-top laser-driven hard x-ray sources with kilohertz repetition rates are an attractive alternative to large-scale accelerator-based systems and have found widespread applications in x-ray studies of ultrafast structural dynamics. Hard x-ray pulses of 100 fs duration have been generated at the Cu K α wavelength with a photon flux of up to 109 photons per pulse into the full solid angle, perfectly synchronized to the sub-100-fs optical pulses from the driving laser system. Based on spontaneous x-ray emission, such sources display a particular noise behavior which impacts the sensitivity of x-ray diffraction experiments. We present a detailed analysis of the photon statistics and temporal fluctuations of the x-ray flux, together with experimental strategies to optimize the sensitivity of optical pump/x-ray probe experiments. We demonstrate measurements close to the shot-noise limit of the x-ray source.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Condensed Matter Highlight A film of picosecond vibrations of a film

Time-domain experiments on solid-state dynamics at the fastest time-scales are typically performed using all optical techniques. These experiments have been made possible by, and have driven significant advances in, pulsed laser technology. Since optical techniques only indirectly probe structure, there is a significant scientific motivation for using higher spatial resolution probes such as X-...

متن کامل

Single-shot femtosecond x-ray holography using extended references.

In the context of x-ray lensless imaging, we present a recent approach for Fourier transform holography based on the use of extended references. Major advances shown here rely on a high signal efficiency and on the direct image reconstruction of the object performed by a simple linear derivative. Moreover, the extended holographic reference is easy to manufacture and can be applied to a variety...

متن کامل

Femtosecond photoelectron diffraction: a new approach to image molecular structure during photochemical reactions

Continuing technical advances in the creation of (sub-) femtosecond VUV and X-ray pulses with Free-Electron Lasers and laser-based high-harmonic-generation sources have created new opportunities for studying ultrafast dynamics during chemical reactions. Here, we present an approach to image the geometric structure of gas-phase molecules with fewfemtosecond temporal and sub-Ångström spatial reso...

متن کامل

A split-beam probe-pump-probe scheme for femtosecond time resolved protein X-ray crystallography

In order to exploit the femtosecond pulse duration of X-ray Free-Electron Lasers (XFEL) operating in the hard X-ray regime for ultrafast time-resolved protein crystallography experiments, critical parameters that determine the crystallographic signal-to-noise (I/σI) must be addressed. For single-crystal studies under low absorbed dose conditions, it has been shown that the intrinsic pulse inten...

متن کامل

Automated identification and classification of single particle serial femtosecond X-ray diffraction data.

The first hard X-ray laser, the Linac Coherent Light Source (LCLS), produces 120 shots per second. Particles injected into the X-ray beam are hit randomly and in unknown orientations by the extremely intense X-ray pulses, where the femtosecond-duration X-ray pulses diffract from the sample before the particle structure is significantly changed even though the sample is ultimately destroyed by t...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:

دوره 4  شماره 

صفحات  -

تاریخ انتشار 2017